This list doesn't include songs on my favorite record, "Graceland" by Paul Simon. In someone else's words:
"Trust me; you are a lesser individual without having heard this album. It is not just a collection of songs; it is an experience." I think words like "lesser individual" are a bit excessive, but the bottom line is: go get yourself a copy.
That being said, in no particular order...
Led Zeppelin - Fool in the Rain Joni Mitchell - Carey Simon and Garfunkel - The Boxer Israel Kamakawiwo'ole - Over the Rainbow / What a Wonderful World Joni Mitchell - All I Want Peter, Paul, and Mary - Puff Leahy - The Call to Dance Medley Mary Bergin - Rileanna - Cinnte Le Dia Rolling Stones - Sympathy for the Devil